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B. 64-bit Machine with 64-bit Version of Word:
Browse to this EndNote folder:

EndNote X6: C:\Program Files (x86)\EndNote X6\Product-Support\CWYW 
EndNote X5: C:\Program Files (x86)\EndNote X5\Product-Support\CWYW
EndNote X4: C:\Program Files (x86)\EndNote X4\Product-Support\CWYW
Copy these files:
EndNote Cwyw.dot
EndNote Cwyw.dotm
EndNote Web Cwyw.dot
EndNote Web Cwyw.dotm
Browse to this destination folder:

EndNote X6: C:\Program Files\Common Files\ResearchSoft\Cwyw\16
EndNote X5: C:\Program Files\Common Files\ResearchSoft\Cwyw\15
EndNote X4: C:\Program Files\Common Files\ResearchSoft\Cwyw\14
Paste the copied files.
Browse to this EndNote folder:

EndNote X6: C:\Program Files (x86)\EndNote X6\Product-Support\CWYW\x64
EndNote X5: C:\Program Files (x86)\EndNote X5\Product-Support\CWYW\x64
EndNote X4: C:\Program Files (x86)\EndNote X4\Product-Support\CWYW\x64
Copy these files:

EndNote Cwyw.dll
ManagedCode.dll
Browse to this destination folder:

EndNote X6: C:\Program Files\Common Files\ResearchSoft\Cwyw\16
EndNote X5: C:\Program Files\Common Files\ResearchSoft\Cwyw\15
EndNote X4: C:\Program Files\Common Files\ResearchSoft\Cwyw\14
Paste the copied files.
Follow the installation steps above.

All currently supported versions of EndNote are 32-bit applications. EndNote when installed on x64 based systems will install by default to:"C:\Program Files (x86)\EndNote (#)" where (#) is the version of EndNote. 重新查看了EndNote主页，X4可以与WIN7 64位兼容，但与64位office 2010不兼容。 LZ只能换32位 office 2010了。 Word Processor Compatibility: EndNote is compatible with the following word processing and text formats: Cite While You Write feature compatible with: Microsoft Word® 2003, 2007 & 2010 (32 bit) Note: Microsoft recommends 32-bit Office 2010 for both 32-bit and 64-bit operating systems. Office 64-bit is optimized for advanced data analysis scenarios that most users don抰 require, and existing 32-bit add-ins are not supported on Office 64-bit.

Overview of Citation Software at MIT: Managing Your References. Endnote, RefWorks and Zotero

There's so many other options out there now...Mendeley, Qigga, etc.