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Economical CO2, SOx, and NOx capture from fossil-fuel utilization with combined renewable hydrogen production and large-scale carbon sequestration Danny Daya, Corresponding Author Contact Information, E-mail The Corresponding Author, Robert J. Evansb, James W. Leec and Don Reicoskyd aEprida, Inc., 6300 Powers Ferry Road, Suite 307, Atlanta, GA 30339, USA bNational Renewable Energy Laboratory, 1617 Cole Blvd, Golden, CO 80401, USA cOak Ridge National Laboratory, 4500N, A16, MS-6194, Oak Ridge, TN 37831, USA dUSDA-Agricultural Research Service, 803 Iowa Avenue, Morris, MN 56267, USA Available online 17 November 2004. Purchase the full-text article References and further reading may be available for this article. To view references and further reading you must purchase this article. Abstract The objective of this project was to investigate and demonstrate production methods at a continuous, bench-scale level and generate sufficient material for an initial evaluation of a potentially profitable method of producing bioenergy and sequestering carbon. The novel process uses agricultural, forestry, and waste biomass to produce hydrogen using pyrolysis and reforming technologies conducted in a 50 kg/h pilot demonstration. The test runs produced a novel, nitrogen-enriched, slow-release, carbon-sequestering fertilizer. Seven kilograms of the material were produced for further plant growth response testing. A pyrolysis temperature profile was discovered that results in a carbon char with an affinity for capturing CO2 through gas phase reaction with mixed nitrogen-carrying nutrient compounds within the pore structures of the carbon char. A bench-scale project demonstrated a continuous process fluidized-bed agglomerating process. The total amount of CO2 sequestration was managed by controlling particle discharge rates based on density. The patent-pending process is particularly applicable to fossil-fuel power plants as it also removes SOx and NOx, does not require ene

Power generation by biomass fuels gasification and its comprehensive utilization is a rising industry. Our company specially recruit Mr. Guo Dezhang, expert and patent owner in this field, to research and design newly type complete set of equipment of biomass gasification power generation in order to reduce the fuel cost for the users and improve the efficiency of energy exchange. According to users needs, safe and reliable computerized controlling system can be designed. For the ash residue of the burned materials, it can be used to produce white carbon black, activated carbon and machine carbon, which can make comprehensive use of recycling energy and helpful to harmonious development of human being and nature.

Producing fuel alcohol via hydrolysis of lignocellulosic biomass leaves a considerable amount of residues waiting for treatment. A study was carried out on the preparation of hydrogen via catalytic gasification of residues from biomass hydrolysis with a novel Ni/modified dolomite binary catalyst, which was prepared by a two-step coprecipitation method and proved available for hydrogen production in terms of both activity and strength. The effects of four operation parameters, that is, the fluidized bed temperature, the catalytic fixed bed temperature, the particle size of the catalyst, and S/B (i.e., the mass ratio of steam to biomass material fed into the fluidized bed per unit time), on hydrogen yield were investigated. The results indicate that hydrogen yield increases with an increase in the temperature of either the fluidized bed or the downstream catalytic fixed bed or the S/B ratio or a reduction in the particle size of the catalyst. The optimum range for each of the four operation parameters from a comprehensive consideration is as follows: 800-850 °C for both the fluidized bed temperature and the catalytic fixed bed temperature, 1.5-2 for the S/B ratio, and 2.0-3.0 mm for the particle size of the catalyst. Furthermore, the gas product from catalytic gasification of residues from biomass hydrolysis contains less CO and CO2 and has a higher H2/CO ratio compared with that of the sawdust. The hydrogen yield of the former is also much higher than that of the latter. These suggest that residues from biomass hydrolysis are an even better gasification material than the original sawdust. This paper provides a novel effective method for modifying the calcined dolomite, which endows the catalyst with satisfactory strength while retaining high activity, and opens a new promising way for utilizing the residues from biomass hydrolysis. Download the full text: PDF | HTML