Impacts of the Fukushima Nuclear Power Plants on Marine Radioactivity - Environmental S... - 0 views
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The impacts on the ocean of releases of radionuclides from the Fukushima Dai-ichi nuclear power plants remain unclear. However, information has been made public regarding the concentrations of radioactive isotopes of iodine and cesium in ocean water near the discharge point. These data allow us to draw some basic conclusions about the relative levels of radionuclides released which can be compared to prior ocean studies and be used to address dose consequences as discussed by Garnier-Laplace et al. in this journal.(1) The data show peak ocean discharges in early April, one month after the earthquake and a factor of 1000 decrease in the month following. Interestingly, the concentrations through the end of July remain higher than expected implying continued releases from the reactors or other contaminated sources, such as groundwater or coastal sediments. By July, levels of 137Cs are still more than 10 000 times higher than levels measured in 2010 in the coastal waters off Japan. Although some radionuclides are significantly elevated, dose calculations suggest minimal impact on marine biota or humans due to direct exposure in surrounding ocean waters, though considerations for biological uptake and consumption of seafood are discussed and further study is warranted.
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there was no large explosive release of core reactor material, so most of the isotopes reported to have spread thus far via atmospheric fallout are primarily the radioactive gases plus fission products such as cesium, which are volatilized at the high temperatures in the reactor core, or during explosions and fires. However, some nonvolatile activation products and fuel rod materials may have been released when the corrosive brines and acidic waters used to cool the reactors interacted with the ruptured fuel rods, carrying radioactive materials into the ground and ocean. The full magnitude of the release has not been well documented, nor is there data on many of the possible isotopes released, but we do have significant information on the concentration of several isotopes of Cs and I in the ocean near the release point which have been publically available since shortly after the accident started.
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We present a comparison of selected data made publicly available from a Japanese company and agencies and compare these to prior published radionuclide concentrations in the oceans. The primary sources included TEPCO (Tokyo Electric Power Company), which reported data in regular press releases(3) and are compiled here (Supporting Information Table S1). These TEPCO data were obtained by initially sampling 500 mL surface ocean water from shore and direct counting on high-purity germanium gamma detectors for 15 min at laboratories at the Fukushima Dai-ni NPPs. They reported initially results for 131I (t1/2 = 8.02 days), 134Cs (t1/2 = 2.065 years) and 137Cs (t1/2 = 30.07 years). Data from MEXT (Ministry of Education, Culture, Sports, Science and Technology—Japan) were also released on a public Web site(4) and are based on similar direct counting methods. In general MEXT data were obtained by sampling 2000 mL seawater and direct counting on high-purity germanium gamma detectors for 1 h in a 2 L Marinelli beaker at laboratories in the Japan Atomic Energy Agency. The detection limit of 137Cs measurements are about 20 000 Bq m–3 for TEPCO data and 10 000 Bq m–3 for MEXT data, respectively. These measurements were conducted based on a guideline described by MEXT.(5) Both sources are considered reliable given the common activity ratios and prior studies and expertise evident by several Japanese groups involved in making these measurements. The purpose of these early monitoring activities was out of concern for immediate health effects, and thus were often reported relative to statutory limits adopted by Japanese authorities, and thus not in concentration units (reported as scaling factors above “normal”). Here we convert values from both sources to radionuclide activity units common to prior ocean studies of fallout in the ocean (Bq m–3) for ease of comparison to previously published data.
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